Lukas Wacker
Datos Biográficos
| ID | 2470367 |
|---|---|
| NOMBRE | Lukas Wacker |
| NOMBRES | Lukas |
| APELLIDO | Wacker |
| FIRMA | WACKER L |
| AFILIACIONES | ETH Zurich |
| ORCID | 0000-0002-8215-2678 |
| VERIFICADO | Sí |
| TOTAL DE OBRAS | 63 |
| TOTAL DE CITAS | 1500 |
| TOTAL COMO AUTOR | 63 |
| TOTAL COMO EDITOR | 0 |
| PRIMER AÑO DE PUBLICACIÓN | 2007 |
| AÑO MÁS RECIENTE DE PUBLICACIÓN | 2026 |
| ÍNDICE H | 11 |
An absolutely dated mid-Holocene English yew chronology offers new opportunities for archaeological and palaeoenvironmental research
Research on Holocene climate variability and human history greatly benefits from annually resolved and absolutely dated tree-ring chronologies. The quality and quantity of such records, however, decline back in time, with little tree-ring evidence available for the Early and Middle Holocene. Here, we present a tree-ring width (TRW) chronology from 100 subfossil yews ( Taxus baccata L.) excavated from peat-rich soils in the Fenland region of easte…
Multi-Proxy Tree-Ring Dating during the Younger Dryas
The world's longest tree-ring chronology comprises thousands of oak and pine series from Germany and continuously covers the Holocene back to 12,325 cal BP. A lack of relict wood from the Younger Dryas cold reversal ca. 12,900–11,700 cal BP, however, challenges the extension of this absolutely dated ring width record further back in time. Here, we combine 646 high-resolution stable oxygen isotope and 795 radiocarbon measurements from subfossil pi…
Pollen 14 C dating compared with established dating methods
Radiocarbon ( 14 C) dating is a powerful tool for establishing reliable chronologies for proxy records recovered from environmental archives, including lacustrine sediments. However, lacustrine sediments are often limited with respect to availability of material such as terrestrial macrofossils that are traditionally targeted for 14 C dating. Flow cytometry, in combination with physicochemical preprocessing, is an emerging technique for the isola…
Towards online ramped oxidation (ORO)-AMS for thermal dissection and serial radiocarbon analysis of complex organic matter
By constraining organic carbon (OC) turnover times and ages, radiocarbon ( 14 C) analysis has become a crucial tool to study the global carbon cycle. However, commonly used “bulk” measurements yield average turnover times, masking age variability within complex OC mixtures. One method to unravel intra-sample age distributions is ramped oxidation, in which OC is oxidized with the aid of oxygen at increasing temperatures. The resulting CO 2 is coll…
Radiocarbon measurements of dissolved inorganic carbon (DIC) in sediment porewater and seawater at AWI Micadas
Radiocarbon ( 14 C) measurements on dissolved inorganic carbon (DIC) are a powerful tool to trace water masses and carbon cycling in the ocean. Existing methodologies to determine the 14 C content of seawater DIC requires large volumes of sample (usually >100 mL) and specialized graphitization techniques to achieve the accuracy and precision needed for meaningful data interpretation. The advancement of the CO 2 gas ionization accelerator mass spe…
The Burial from Aleti Tunu Bibi Cave, Atauro Island, East Timor
The Aleti Tunu Bibi cave, located on the small volcanic island of Atauro close to the island of Timor, is a sacred site for the region's inhabitants. The cave's archaeological potential was revealed in 2015 with the discovery of artifacts, rock art depicting marine fauna (mammals and reptiles), human remains, and a few remains of marine and terrestrial fauna. New material discovered in 2017 included sporadic remains of marine fauna, goats and pig…
Lea—a Novel Low Energy Accelerator for 14 C Dating
A newly developed compact AMS, LEA (Low Energy Accelerator), is tested and compared with a state-of-the-art AMS system MICADAS (Mini Carbon Dating System), which has a precision performance of better than 1‰ for modern 14 C. The main difference between these two systems is the acceleration voltage, which has been reduced from 200 kV with the MICADAS system to 50 kV with the LEA system. In order to execute the final performance tests, exactly same…
Safe Preparation and Delivery of Graphite Targets for 14 C Analysis
Nowadays, most radiocarbon ( 14 C) laboratories can reliably avoid and remove any possible sample contamination during the pretreatment of organic samples (e.g., bones, charcoal, or trees) thanks to a series of methods commonly used by the radiocarbon community. However, what about the final step, the storage of graphite? Rarely do the laboratories produce their graphite and ship it as pressed targets to accelerator mass spectrometry (AMS) facili…
A Universal Gas Interface for Simultaneous 14 C and Δ 13 C Measurements
While simultaneous radiocarbon and δ 13 C measurements have been available for organic materials (by accelerator mass spectrometry, AMS, and isotope ratio mass spectrometry, IRMS, respectively), this has not been possible for carbonates until now. Using an existing interface for gas ion source AMS measurements, we developed a prototype for a universal gas interface that allows simultaneous measurement of both carbon isotope ratios from potentiall…
Caveat emptor !—wiggle-matching European wood samples (AD 46–AD 286)
This study suggests that there may be considerable difficulties in providing accurate calendar age estimates in the Roman period in Europe, between ca. AD 60 and ca. AD 230, using the radiocarbon calibration datasets that are currently available. Incorporating the potential for systematic offsets between the measured data and the calibration curve using the ΔR approach suggested by Hogg et al. (2019), only marginally mitigates the biases in calen…
Contrasting paired benthic and planktonic foraminifera radiocarbon ages from Bermuda Rise ODP Site 1063 during Heinrich Stadials 1 and 2
We report 27 planktonic and 21 benthic radiocarbon ages from the subtropical marine sediment core ODP Site 1063 (Bermuda Rise) for the time range between 30 and 14 ka before present. Despite low abundances of benthic specimens, it was possible to measure radiocarbon ages down to ∼10 μg carbon using a MICADAS and the gas ion source developed at ETH Zurich. Based on a tentative radiocarbon–independent age-model we found that the radiocarbon reservo…
Preparation and Handling of Methane for Radiocarbon Analysis at Cologneams
CH 4 is the second most important anthropogenic greenhouse gas and originates from different sources. The use of radiocarbon ( 14 C) analysis of CH 4 opens up the possibility to differentiate geological and agricultural origin. At the CologneAMS facility, the demand for 14 C analysis of CH 4 required the development of a sample handling routine and a vacuum system that converts CH 4 to CO 2 for direct injection of CO 2 into the AMS. We evaluated …
To date or not to date? A comparison of different 14 C pretreatment methods applied to archeological marine shells from Vale Boi (Portugal)
Mollusk shells are often found in archeological sites, given their great preservation potential and high value as a multipurpose resource, and they can often be the only available materials useful for radiocarbon ( 14 C) dating. However, dates obtained from shells are often regarded as less reliable compared to those from bones, wood, or charcoals due to different factors (e.g., Isotope fractionation, reservoir effects etc.). The standard acid et…
Comparability of Radiocarbon Measurements in Dissolved Inorganic Carbon of Seawater Produced at Eth-Zurich
Radiocarbon observations (Δ 14 C) in dissolved inorganic carbon (DIC) of seawater provide useful information about ocean carbon cycling and ocean circulation. To deliver high-quality observations, the Laboratory of Ion Beam Physics (LIP) at ETH-Zurich developed a new simplified method allowing the rapid analysis of radiocarbon in DIC of small seawater samples, which is continually assessed by following internal quality controls. However, a compar…
C Microsample Analysis With Echomicadas Facilities
In 2015, a new accelerator mass spectrometry facility (AMS), the ECHoMICADAS (Environnement, Climat, Homme, MIni CArbon DAting System), was installed in the Laboratoire des Sciences du Climat et de l’Environnement (LSCE). Equipped with a hybrid source, it allows the analysis of solid or gas samples for 14 C measurement. Here, we summarize the equipment surrounding the Gas Interface System (GIS), namely the elemental analyzer (EA), the carbonate h…
Origin and Age of Carbon in the Cellulose of Mid-Latitude Tree Rings
Cellulose of tree rings is often assumed to be predominantly formed by direct assimilation of CO 2 by photosynthesis and consequently can be used to reconstruct past atmospheric 14 C concentrations at annual resolution. Yet little is known about the extent and the age of stored carbon from previous years used in addition to the direct assimilation in tree rings. Here, we studied 14 C in earlywood and latewood cellulose of four different species (…
Development of the Intcal Database
The IntCal family of radiocarbon ( 14 C) calibration curves is based on research spanning more than three decades. The IntCal group have collated the 14 C and calendar age data (mostly derived from primary publications with other types of data and meta-data) and, since 2010, made them available for other sorts of analysis through an open-access database. This has ensured transparency in terms of the data used in the construction of the ratified c…
A Late Holocene climate reconstruction from the high-altitude Lake Gölcük sedimentary records, Isparta (SW Anatolia)
A high-resolution multiproxy lake sediment dataset, comprising lithology, radiography, μXRF elemental, magnetic susceptibility (MS), δ 13 C, and δ 18 O measurements since ca. AD 400 is presented in this study. Changes in lithology, radiography, magnetic susceptibility (MS), δ 13 C, and δ 18 O reflect wet/dry climate periods, whereas variability in log(Ca/K) can reflect warm/cold climate periods. Analyses of the multiproxy results allow the distin…
Holocene deglaciation and glacier readvances on the Fildes Peninsula and King George Island (Isla 25 de Mayo), South Shetland Islands, NW Antarctic Peninsula
To provide insights into glacier-climate dynamics of the South Shetland Islands (SSI), NW Antarctic Peninsula, we present a new deglaciation and readvance model for the Bellingshausen Ice Cap (BIC) on Fildes Peninsula and for King George Island/Isla 25 de Mayo (KGI) ~62°S. Deglaciation on KGI began after c. 15 cal. ka BP and had progressed to within present-day limits on the Fildes Peninsula, its largest ice-free peninsula, by c. 6.6–5.3 cal. ka …
The glacier advance at the onset of the Little Ice Age in the Alps
The term ‘Little Ice Age’ (LIA) is classically used to define a period of repeated and extensive glacier advances during the last millennium. In the meanwhile, this term is also used to address the period of relatively low temperatures between the Medieval Climate Anomaly (MCA), or Medieval Warm Period, and present-day warming. The end of the LIA is generally set to the mid or late 1800s CE, however, the published onset dates of the LIA are more …
Premature Oxidation During Argon Plasma Cleaning of Water-Rich Radiocarbon Samples
Plasma oxidation for 14 C sampling utilizes low-pressure (133 Pa), low-energy ( 2 -plasmas generating CO 2 for AMS dating. O 2 -plasmas on empty chambers remove organic contamination. When clean, a new specimen is inserted and Ar-plasmas dislodge adsorbed atmospheric CO 2 from surfaces. Finally, O 2 -plasmas oxidize organic materials to CO 2 for AMS analysis. During some Ar-plasmas we observed anomalous pressure increases and unexpectedly high CO…
Hydrographic shifts south of Australia over the last deglaciation and possible interhemispheric linkages
Northern and southern hemispheric influences—particularly changes in Southern Hemisphere westerly winds (SSW) and Southern Ocean ventilation—triggered the stepwise atmospheric CO 2 increase that accompanied the last deglaciation. One approach for gaining potential insights into past changes in SWW/CO 2 upwelling is to reconstruct the positions of the northern oceanic fronts associated with the Antarctic Circumpolar Current. Using two deep-sea cor…
Re-dating the Lower Pecos Canyonlands SMM (Skiles) mummy burial, dating a red-colored deerskin strap
Radiocarbon Protocols and First Intercomparison Results From the Chronos 14 Carbon-Cycle Facility, University of New South Wales, Sydney, Australia
The Chronos 14 Carbon-Cycle Facility is a new radiocarbon laboratory at the University of New South Wales, Australia. Built around an Ionplus 200 kV MIni-CArbon DAting System (MICADAS) Accelerator Mass Spectrometer (AMS) installed in October 2019, the facility was established to address major challenges in the Earth, Environmental and Archaeological sciences. Here we report an overview of the Chronos facility, the pretreatment methods currently e…
Gas Ion Source Performance of the Environmicadas at Hekal Laboratory, Debrecen, Hungary
A coupled accelerator mass spectrometer–gas interface system has been successfully operating at the Hertelendi Laboratory of Environmental Studies, Debrecen, Hungary, since 2013. Over the last 6 years more than 500 gas targets were measured below 100 μg carbon content for carbon isotopic composition. The system was tested with blanks, OxII, IAEA-C1, IAEA-C2, and IAEA-C7 standards. The performance of our instrumentation shows good agreement with o…
The IntCal20 Northern Hemisphere Radiocarbon Age Calibration Curve (0–55 cal kBP)
Radiocarbon ( 14 C) ages cannot provide absolutely dated chronologies for archaeological or paleoenvironmental studies directly but must be converted to calendar age equivalents using a calibration curve compensating for fluctuations in atmospheric 14 C concentration. Although calibration curves are constructed from independently dated archives, they invariably require revision as new data become available and our understanding of the Earth syste…
SHCal20 Southern Hemisphere Calibration, 0–55,000 Years cal BP
Early researchers of radiocarbon levels in Southern Hemisphere tree rings identified a variable North-South hemispheric offset, necessitating construction of a separate radiocarbon calibration curve for the South. We present here SHCal20, a revised calibration curve from 0–55,000 cal BP, based upon SHCal13 and fortified by the addition of 14 new tree-ring data sets in the 2140–0, 3520–3453, 3608–3590 and 13,140–11,375 cal BP time intervals. We de…
Alternative Methods for Cellulose Preparation for AMS Measurement
The main methods applied to clean plant material for radiocarbon dating are not compound-specific and generally remove only the easily exchangeable components by an acid-base-acid sequence and additional optional steps like Soxhlet extraction to remove resins and oxidative bleaching with NaClO 2 . The products are normally clean enough for standard 14 C measurement, but in some cases it is desirable to have pure cellulose, which remains unchanged…
C Analysis and Sample Preparation at the New Bern Laboratory for the Analysis of Radiocarbon with AMS (Lara)
The University of Bern has set up the new Laboratory for the Analysis of Radiocarbon with AMS (LARA) equipped with an accelerator mass spectrometer (AMS) MICADAS (MIni CArbon Dating System) to continue its long history of 14 C analysis based on conventional counting. The new laboratory is designated to provide routine 14 C dating for archaeology, climate research, and other disciplines at the University of Bern and to develop new analytical syste…
Dating Bones near the Limit of the Radiocarbon Dating Method
Preparation of bone material for radiocarbon dating is still a subject of investigation. In the past, the most problematic ages appeared to be the very old bones, i.e. those with ages close to the limit of the dating method. Development of preparative methods requires sufficient amounts of bone material as well as the possibility of verification of the ages. In the peat section at Niederweningen, ZH Switzerland, numerous bones of mammoth and othe…
The New Zealand Kauri ( Agathis Australis ) Research Project
Wc describe here the New Zealand kauri ( Agathis australis ) Younger Dryas (YD) research project, which aims to undertake Δ 14 C analysis of ∼140 decadal floating wood samples spanning the time interval ∼13.1–11.7 kyr cal BP. We report 14 C intercomparison measurements being undertaken by the carbon dating laboratories at University of Waikato (Wk), University of California at Irvine (UCI), and University of Oxford (OxA). The Wk, UCI, and OxA lab…
Roman Ruins as an Experiment for Radiocarbon Dating of Mortar
The remains of Vindonissa, the Roman legionary camp in Switzerland, have been the subject of extensive archaeological studies. Knowledge of the building time plays a role in reconstructions of the history of this site. We radiocarbon dated mortar samples selected from one of the Roman monuments (Westtor) as well as a nearby Medieval monastery. 14 C ages obtained on the first fraction and second fraction of very short dissolution appear close to t…
Radiocarbon Protocols and First Intercomparison Results From the Chronos 14 Carbon-Cycle Facility, University of New South Wales, Sydney, Australia
The Chronos 14 Carbon-Cycle Facility is a new radiocarbon laboratory at the University of New South Wales, Australia. Built around an Ionplus 200 kV MIni-CArbon DAting System (MICADAS) Accelerator Mass Spectrometer (AMS) installed in October 2019, the facility was established to address major challenges in the Earth, Environmental and Archaeological sciences. Here we report an overview of the Chronos facility, the pretreatment methods currently e…
Decadally Resolved Lateglacial Radiocarbon Evidence from New Zealand Kauri
The Last Glacial–Interglacial Transition (LGIT; 15,000–11,000 cal BP) was characterized by complex spatiotemporal patterns of climate change, with numerous studies requiring accurate chronological control to decipher leads from lags in global paleoclimatic, paleoenvironmental, and archaeological records. However, close scrutiny of the few available tree-ring chronologies and radiocarbon-dated sequences composing the IntCal13 14 C calibration curv…
IntCal20 Tree Rings
We undertook a strengths, weaknesses, opportunities, and threats (SWOT) analysis of Northern Hemisphere tree-ring datasets included in IntCal20 in order to evaluate their strategic fit with the demands of archaeological users. Case studies on wiggle-matching single tree rings from timbers in historic buildings and Bayesian modeling of series of results on archaeological samples from Neolithic long barrows in central-southern England exemplify the…
Annual Variation in Atmospheric 14 C Between 1700 BC and 1480 BC
In 2018 Pearson et al. published a new sequence of annual radiocarbon ( 14 C) data derived from oak ( Quercus sp.) trees from Northern Ireland and bristlecone pine ( Pinus longaeva ) from North America across the period 1700–1500 BC. The study indicated that the more highly resolved shape of an annually based calibration dataset could improve the accuracy of 14 C calibration during this period. This finding had implications for the controversial …
Findings from an in-Depth Annual Tree-Ring Radiocarbon Intercomparison
The radiocarbon ( 14 C) calibration curve so far contains annually resolved data only for a short period of time. With accelerator mass spectrometry (AMS) matching the precision of decay counting, it is now possible to efficiently produce large datasets of annual resolution for calibration purposes using small amounts of wood. The radiocarbon intercomparison on single-year tree-ring samples presented here is the first to investigate specifically …
A Chronology of the Pre-Columbian Paracas and Nasca Cultures in South Peru Based on AMS 14 C Dating
The people of the Paracas and Nasca cultures, the creators of the famous geoglyphs, lived in the desert of the southern coast of Peru between about 800 BC and AD 650. The archaeological chronology of these cultures has been based almost exclusively on a sequence of ceramic styles. The absolute dating of some of the style phases was supported by a few radiocarbon dates (Rowe 1967). Here, we present an absolute chronology of the Paracas and Nasca c…
A New Annual 14 C Dataset for Calibrating the Thera Eruption
Annually resolved tree-ring samples of the time period 1625–1510 BCE were analyzed from the German oak tree-ring chronology. Blocks of the same tree rings were previously used to generate IntCal calibration data. The new dataset shows an offset to the calibration data IntCal13 of 24 years and resembles annual data for the same time period derived from tree-ring records in other growth locations. A subset of samples of the period 1625–1585 BCE was…
Quality Dating
Advances in accelerator mass spectrometry have resulted in an unprecedented amount of new high-precision radiocarbon ( 14 C) -dates, some of which will redefine the international 14 C calibration curves (IntCal and SHCal). Often these datasets are unaccompanied by detailed quality insurances in place at the laboratory, questioning whether the 14 C structure is real, a result of a laboratory variation or measurement-scatter. A handful of intercomp…
Combined 14 C Analysis of Canvas and Organic Binder for Dating a Painting
The use of accelerator mass spectrometry (AMS) for age determinations of paintings is growing due to decreasing sample size requirements. However, as only the support material is usually dated, the validity of the results may be questioned. This work describes a novel sampling and preparation technique for dating the natural organic binder using radiocarbon ( 14 C) AMS. In the particular case of oil paintings, the natural oil used has a high prob…
Single-Year German oak and Californian Bristlecone Pine 14 C Data at the Beginning of the Hallstatt Plateau from 856 BC to 626 BC
As part of the ongoing effort to improve the Northern Hemisphere radiocarbon ( 14 C) calibration curve, this study investigates the period of 856 BC to 626 BC (2805–2575 yr BP) with a total of 403 single-year 14 C measurements. In this age range, IntCal13 was constructed largely from German and Irish oak as well as Californian bristlecone pine 14 C dates, with most samples measured with a 10-yr resolution. The new data presented here is the first…
Rapid 14 C Analysis of Dissolved Organic Carbon in Non-Saline Waters
The radiocarbon content of dissolved organic carbon (DOC) in rivers, lakes, and other non-saline waters can provide valuable information on carbon cycling dynamics in the environment. DOC is typically prepared for 14 C analysis by accelerator mass spectrometry (AMS) either by ultraviolet (UV) oxidation or by freeze-drying and sealed tube combustion. We present here a new method for the rapid analysis of 14 C of DOC using wet chemical oxidation (W…
Illuminating Intcal During the Younger Dryas
As the worldwide standard for radiocarbon ( 14 C) dating over the past ca. 50,000 years, the International Calibration Curve (IntCal) is continuously improving towards higher resolution and replication. Tree-ring-based 14 C measurements provide absolute dating throughout most of the Holocene, although high-precision data are limited for the Younger Dryas interval and farther back in time. Here, we describe the dendrochronological characteristics …
Gas Ion Source Performance of the Environmicadas at Hekal Laboratory, Debrecen, Hungary
A coupled accelerator mass spectrometer–gas interface system has been successfully operating at the Hertelendi Laboratory of Environmental Studies, Debrecen, Hungary, since 2013. Over the last 6 years more than 500 gas targets were measured below 100 μg carbon content for carbon isotopic composition. The system was tested with blanks, OxII, IAEA-C1, IAEA-C2, and IAEA-C7 standards. The performance of our instrumentation shows good agreement with o…
High Precision 14 C Analysis in Small Seawater Samples
A new method to extract CO 2 in seawater samples for the determination of F 14 C has been developed in the Laboratory of Ion Beam Physics at ETH Zurich. The setup consists of an automated sampler designed to extract dissolved inorganic carbon (DIC) from 7 samples in a row, by flushing the seawater with He gas to extract CO 2 . The fully automated method is controlled via a LabVIEW program that runs through all consecutive steps: catalyst precondi…
Radiocarbon Dating of Small-sized Foraminifer Samples
Radiocarbon ( 14 C) can be used to build absolute chronologies and reconstruct ocean ventilation over the last 40 ka. Sample size requirements have restricted 14 C measurements in marine cores with low foraminifer content, impeding 14 C-based studies focused on abrupt climate events. Recent developments have demonstrated that small-sized foraminifer samples can now be dated using a gas introduction system at the cost of a small decrease in precis…
C Blank Assessment in Small-Scale Compound-Specific Radiocarbon Analysis of Lipid Biomarkers and Lignin Phenols
Compound-specific radiocarbon ( 14 C) dating often requires working with small samples of 14 C) and the mass of the procedural blanks introduced during the preparation procedures of lipid biomarkers (i.e. n -alkanoic acids) and lignin phenols. We isolated differently sized aliquots (6–151 μgC) of n -alkanoic acids and lignin phenols obtained from standard materials with known F 14 C values. Each compound class was extracted from two standard mate…
Status Report on the Sample Preparation Laboratory for Radiocarbon Dating at the New Bucharest Roams Center
The accelerator mass spectrometry (AMS) center at Horia Hulubei National Institute for R&D in Physics and Nuclear Engineering, Bucharest, is based on the latest-generation 1 MV Tandetron ® accelerator, produced by High Voltage Engineering Europa (HVEE), The Netherlands. The AMS center became fully functional at the start of 2013, and at the end of 2015 the laboratory established the RoAMS international code and it was added to the list of AMS lab…
Online 13 C and 14 C Gas Measurements by EA-IRMS–AMS at ETH Zürich
Studies using carbon isotopes to understand the global carbon cycle are critical to identify and quantify sources, sinks, and processes and how humans may impact them. 13 C and 14 C are routinely measured individually; however, there is a need to develop instrumentation that can perform concurrent online analyses that can generate rich data sets conveniently and efficiently. To satisfy these requirements, we coupled an elemental analyzer to a sta…
Dating methods and geomorphic evidence of palaeoenvironmental changes at the eastern margin of the South Peruvian coastal desert (14°30′S) before and during the Little Ice Age
A Chronology of the Pre-Columbian Paracas and Nasca Cultures in South Peru Based on AMS 14 C Dating
The people of the Paracas and Nasca cultures, the creators of the famous geoglyphs, lived in the desert of the southern coast of Peru between about 800 BC and AD 650. The archaeological chronology of these cultures has been based almost exclusively on a sequence of ceramic styles. The absolute dating of some of the style phases was supported by a few radiocarbon dates (Rowe 1967). Here, we present an absolute chronology of the Paracas and Nasca c…
Dating Bones near the Limit of the Radiocarbon Dating Method
Preparation of bone material for radiocarbon dating is still a subject of investigation. In the past, the most problematic ages appeared to be the very old bones, i.e. those with ages close to the limit of the dating method. Development of preparative methods requires sufficient amounts of bone material as well as the possibility of verification of the ages. In the peat section at Niederweningen, ZH Switzerland, numerous bones of mammoth and othe…
A revolutionary graphitisation system
Bats
Alternative Methods for Cellulose Preparation for AMS Measurement
The main methods applied to clean plant material for radiocarbon dating are not compound-specific and generally remove only the easily exchangeable components by an acid-base-acid sequence and additional optional steps like Soxhlet extraction to remove resins and oxidative bleaching with NaClO 2 . The products are normally clean enough for standard 14 C measurement, but in some cases it is desirable to have pure cellulose, which remains unchanged…
Towards On-Line 14 C Analysis of Carbonaceous Aerosol Fractions
Atmospheric carbonaceous aerosol is traditionally divided into organic carbon (OC) and elemental carbon (EC). Their respective carbon amounts are usually analyzed by means of an OC/EC analyzer and their fossil and non-fossil origins can be determined by radiocarbon analysis, which has proven to be a powerful tool for carbonaceous aerosol source apportionment. Thus far, separation of OC and EC has been performed off-line by manual and time-consumi…
Anomalous Radiocarbon Ages Found in Campanian Ignimbrite Deposit of the Mediterranean Deep-Sea Core CT85-5
A detailed radiocarbon chronology has been established for the deep-sea core CT85-5 from the Tyrrhenian Sea. This chronology, which is based on the analysis of foraminifera shells, shows a set of reversed 14 C ages for sediments deposited during the eruption of the Campanian Ignimbrite (∼40 ka cal BP). The anomalous young 14 C ages coincide with elevated concentrations of 10 Bc measured in the same core. Although reversals in 14 C ages have been …
Roman Ruins as an Experiment for Radiocarbon Dating of Mortar
The remains of Vindonissa, the Roman legionary camp in Switzerland, have been the subject of extensive archaeological studies. Knowledge of the building time plays a role in reconstructions of the history of this site. We radiocarbon dated mortar samples selected from one of the Roman monuments (Westtor) as well as a nearby Medieval monastery. 14 C ages obtained on the first fraction and second fraction of very short dissolution appear close to t…
Mams – A new AMS facility at the Curt-Engelhorn-Centre for Achaeometry, Mannheim, Germany
Microgram-Level Radiocarbon Determination of Carbonaceous Particles in Firn and Ice Samples
Carbonaceous particles that comprise organic carbon (OC) and elemental carbon (EC) are of increasing interest in climate research because of their influence on the radiation balance of the Earth. The radiocarbon determination of particulate OC and EC extracted from ice cores provides a powerful tool to reconstruct the long-term natural and anthropogenic emissions of carbonaceous particles. However, this 14 C-based source apportionment method has …
The New Zealand Kauri ( Agathis Australis ) Research Project
Wc describe here the New Zealand kauri ( Agathis australis ) Younger Dryas (YD) research project, which aims to undertake Δ 14 C analysis of ∼140 decadal floating wood samples spanning the time interval ∼13.1–11.7 kyr cal BP. We report 14 C intercomparison measurements being undertaken by the carbon dating laboratories at University of Waikato (Wk), University of California at Irvine (UCI), and University of Oxford (OxA). The Wk, UCI, and OxA lab…
C Analysis and Sample Preparation at the New Bern Laboratory for the Analysis of Radiocarbon with AMS (Lara)
The University of Bern has set up the new Laboratory for the Analysis of Radiocarbon with AMS (LARA) equipped with an accelerator mass spectrometer (AMS) MICADAS (MIni CArbon Dating System) to continue its long history of 14 C analysis based on conventional counting. The new laboratory is designated to provide routine 14 C dating for archaeology, climate research, and other disciplines at the University of Bern and to develop new analytical syste…
Cooling and societal change during the Late Antique Little Ice Age from 536 to around 660 AD
Rapid 14 C Analysis of Dissolved Organic Carbon in Non-Saline Waters
The radiocarbon content of dissolved organic carbon (DOC) in rivers, lakes, and other non-saline waters can provide valuable information on carbon cycling dynamics in the environment. DOC is typically prepared for 14 C analysis by accelerator mass spectrometry (AMS) either by ultraviolet (UV) oxidation or by freeze-drying and sealed tube combustion. We present here a new method for the rapid analysis of 14 C of DOC using wet chemical oxidation (W…
C Contamination Testing in Natural Abundance Laboratories
Substances enriched with radiocarbon can easily contaminate samples and laboratories used for natural abundance measurements. We have developed a new method using wet chemical oxidation for swabbing laboratories and equipment to test for 14 C contamination. Here, we report the findings of 18 months’ work and more than 800 tests covering studies at multiple locations. Evidence of past and current use of enriched 14 C was found at all but one locat…
Decadally Resolved Lateglacial Radiocarbon Evidence from New Zealand Kauri
The Last Glacial–Interglacial Transition (LGIT; 15,000–11,000 cal BP) was characterized by complex spatiotemporal patterns of climate change, with numerous studies requiring accurate chronological control to decipher leads from lags in global paleoclimatic, paleoenvironmental, and archaeological records. However, close scrutiny of the few available tree-ring chronologies and radiocarbon-dated sequences composing the IntCal13 14 C calibration curv…
From medieval land clearing to industrial development
The Joux Valley (Swiss Jura Mountains) has a rather unusual history of human occupation, characterized by tardive but extensive settlement since the Late Middle Ages, followed by an intensive period of industrial development. To estimate the links between human activities and environmental consequences, sediment cores were retrieved in Lake Joux and submitted to a multiproxy analysis (high-resolution photographs, magnetic susceptibility, density,…
Speed Dating
Radiocarbon measurements in tree rings can be used to estimate atmospheric 14 C concentration and thereby used to create a 14 C calibration curve. When wood is discovered in construction sites, rivers, buildings, and lake sediments, it is unclear if the wood could fill gaps in the 14 C calibration curve or if the wood is of historical interest until the age is determined by dendrochronology or 14 C dating. However, dendrochronological dating is s…
Online 13 C and 14 C Gas Measurements by EA-IRMS–AMS at ETH Zürich
Studies using carbon isotopes to understand the global carbon cycle are critical to identify and quantify sources, sinks, and processes and how humans may impact them. 13 C and 14 C are routinely measured individually; however, there is a need to develop instrumentation that can perform concurrent online analyses that can generate rich data sets conveniently and efficiently. To satisfy these requirements, we coupled an elemental analyzer to a sta…
Combined 14 C Analysis of Canvas and Organic Binder for Dating a Painting
The use of accelerator mass spectrometry (AMS) for age determinations of paintings is growing due to decreasing sample size requirements. However, as only the support material is usually dated, the validity of the results may be questioned. This work describes a novel sampling and preparation technique for dating the natural organic binder using radiocarbon ( 14 C) AMS. In the particular case of oil paintings, the natural oil used has a high prob…
Radiocarbon dating a pictograph at Medicine Lodge Creek, Wyoming
Wyoming State Parks recovered a large chunk of the Medicine Lodge Creek Archaeological Site cliff wall, which had fallen away, with rock paintings on it. A sample from one of the paintings was dated to 800 BP with the Plasma Oxidation dating method. Comparison to regional sites suggests the dated painting is part of the Foothills Abstract tradition or a variant of the Columbia Plateau tradition
Permafrost-carbon mobilization in Beringia caused by deglacial meltwater runoff, sea-level rise and warming
During the last deglaciation (18–8 kyr BP), shelf flooding and warming presumably led to a large-scale decomposition of permafrost soils in the mid-to-high latitudes of the Northern Hemisphere. Microbial degradation of old organic matter released from the decomposing permafrost potentially contributed to the deglacial rise in atmospheric CO 2 and also to the declining atmospheric radiocarbon contents (Δ 14 C). The significance of permafrost for t…
Status Report on the Sample Preparation Laboratory for Radiocarbon Dating at the New Bucharest Roams Center
The accelerator mass spectrometry (AMS) center at Horia Hulubei National Institute for R&D in Physics and Nuclear Engineering, Bucharest, is based on the latest-generation 1 MV Tandetron ® accelerator, produced by High Voltage Engineering Europa (HVEE), The Netherlands. The AMS center became fully functional at the start of 2013, and at the end of 2015 the laboratory established the RoAMS international code and it was added to the list of AMS lab…
Initial Upper Palaeolithic Homo sapiens from Bacho Kiro Cave, Bulgaria
Radiocarbon dating (42 obras) · Geology (41 obras) · Archaeology and ancient environmental studies (37 obras) · Archaeology (33 obras) · Geology and Paleoclimatology Research (33 obras) · Geography (30 obras) · Chemistry (25 obras) · Paleontology (21 obras) · Accelerator mass spectrometry (18 obras) · Environmental Science (17 obras)