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Evaluating the potential of iron-based interventions in methane reduction and climate mitigation

Bibliographic Data

ID15545844
AuthorsDaphne Meidan (0000-0001-7746-4979, Atkins (United States)), Qinyi Li (0009-0008-7438-4461, Shandong University), Carlos A Cuevas (0000-0002-5998-9963, Consejo Superior de Investigaciones Científicas), Scott Doney (0000-0002-3683-2437, University of Virginia), Scott C Doney, Rafael P Fernández (0000-0002-4114-5500, Consejo Nacional de Investigaciones Científicas y Técnicas), Maarten M J W van Herpen (0000-0003-0653-9050, Acacia Pharma (United Kingdom)), Matthew S Johnson (0000-0001-6029-896X, University of Copenhagen), Douglas E Kinnison (0000-0002-3418-0834, NSF National Center for Atmospheric Research), Longlei Li (Cornell University), Douglas S Hamilton (0000-0002-8171-5723, North Carolina State University), Alfonso Saiz‐Lopez (0000-0002-0060-1581, Comunidad de Madrid), Alfonso Saiz-Lopez, Peter Hess (0000-0003-2439-3796, Cornell University), N M Mahowald (0000-0002-2873-997X, Cornell University, corresponding author)
Year2024
Volume19
Issue5
Pages054023-054023
Publication date2024-04-11
Peer ReviewedYes
Open AccessYes
TypeARTICLE
VenueEnvironmental Research Letters (JOURNAL)
Journal identifiersISSN: 1748-9326 • E-ISSN: 1748-9326
PublisherIOP Publishing (PUBLISHER • GB)
DOI10.1088/1748-9326/ad3d72
OpenAlexW4394710063
LanguageEN
Citations received1
References cited57

Keeping global surface temperatures below international climate targets will require substantial measures to control atmospheric CO 2 and CH 4 concentrations. Recent studies have focused on interventions to decrease CH 4 through enhanced atmospheric oxidation. Here for the first time using a set of models, we evaluate the effect of adding iron aerosols to the atmosphere to enhance molecular chlorine production, and thus enhance the atmospheric oxidation of methane and reduce its concentration. Using different iron emission sensitivity scenarios, we examine the potential role and impact of enhanced iron emissions on direct interactions with solar radiation, and on the chemical and radiative response of methane. Our results show that the impact of iron emissions on CH 4 depends sensitively on the location of the iron emissions. In all emission regions there is a threshold in the amount of iron that must be added to remove methane. Below this threshold CH 4 increases. Even once that threshold is reached, the iron-aerosol driven chlorine-enhanced impacts on climate are complex. The radiative forcing of both methane and ozone are decreased in the most efficient regions but the direct effect due to the addition of absorbing iron aerosols tends to warm the planet. Adding any anthropogenic aerosol may also cool the planet due to aerosol cloud interactions, although these are very uncertain, and here we focus on the unique properties of adding iron aerosols. If the added emissions have a similar distribution as current shipping emissions, our study shows that the amount of iron aerosols that must be added before methane decreases is 2.5 times the current shipping emissions of iron aerosols, or 6 Tg Fe yr −1 in the most ideal case examined here. Our study suggests that the photoactive fraction of iron aerosols is a key variable controlling the impact of iron additions and poorly understood. More studies of the sensitivity of when, where and how iron aerosols are added should be conducted. Before seriously considering this method, additional impacts on the atmospheric chemistry, climate, environmental impacts and air pollution should be carefully assessed in future studies since they are likely to be important

Biology · Climate change · Climatology · Economics · Methane · Natural resource economics · Reduction (mathematics · Atmospheric and Environmental Gas Dynamics · Environmental Science · Mathematics · Ecology · Geology

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Unique citing works1
Citations per year0,5
Citation span2024 - 2024 (1)
Citation velocityrecent
Highly citedNo
Citation typesNeutral: 1

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