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Temporal and spatial variability in the aviation NO x -related O 3 impact

Bibliographic Data

ID15549408
AuthorsChristopher K Gilmore (American Institute of Aeronautics and Astronautics), Steven R H Barrett (0000-0002-4642-9545, American Institute of Aeronautics and Astronautics, corresponding author), Jamin Koo (0000-0003-4299-1546, Massachusetts Institute of Technology), Qiqi Wang (0000-0001-8633-1342, Massachusetts Institute of Technology)
Year2013
Volume8
Issue3
Pages034027-034027
Publication date2013-09-01
Open AccessYes
TypeARTICLE
VenueEnvironmental Research Letters (JOURNAL)
Journal identifiersISSN: 1748-9326 • E-ISSN: 1748-9326
PublisherIOP Publishing (PUBLISHER • GB)
DOI10.1088/1748-9326/8/3/034027
OpenAlexW2096580230
LanguageEN
Citations received2
References cited22

Aviation NO _x emissions promote tropospheric ozone formation, which is linked to climate warming and adverse health effects. Modeling studies have quantified the relative impact of aviation NO _x on O _3 in large geographic regions. As these studies have applied forward modeling techniques, it has not been possible to attribute O _3 formation to individual flights. Here we apply the adjoint of the global chemistry–transport model GEOS-Chem to assess the temporal and spatial variability in O _3 production due to aviation NO _x emissions, which is the first application of an adjoint to this problem. We find that total aviation NO _x emitted in October causes 40% more O _3 than in April and that Pacific aviation emissions could cause 4–5 times more tropospheric O _3 per unit NO _x than European or North American emissions. Using this sensitivity approach, the O _3 burden attributable to 83 000 unique scheduled civil flights is computed individually. We find that the ten highest total O _3 -producing flights have origins or destinations in New Zealand or Australia. The top ranked O _3 -producing flights normalized by fuel burn cause 157 times more normalized O _3 formation than the bottom ranked ones. These results show significant spatial and temporal heterogeneity in environmental impacts of aviation NO _x emissions

Atmospheric sciences · Aviation · Civil aviation · Climatology · Combustion · Geography · Meteorology · NOx · Ozone · Troposphere · Tropospheric ozone · Advanced Aircraft Design and Technologies · Air Quality and Health Impacts · Chemistry · Engineering · Environmental Science · Vehicle emissions and performance · Aerospace Engineering · Geology

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    Open Access•Carla Grobler, Philip J Wolfe et al.•Environmental Research Letters•2019

  • Lung Cancer, Cardiopulmonary Mortality, and Long-term Exposure to Fine Particulate Air Pollution

    C Arden Pope, C Arden Pope III•JAMA•2002

  • Reduction in Fine Particulate Air Pollution and Mortality

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Citations per year0.29
Citation span2019 - 2024 (6)
Highly citedNo

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