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Anomalous 14 C Enrichments in the Eastern UK Coastal Environment

Bibliographic Data

ID9241990
AuthorsGraham K P Muir, Gordon Cook (0000-0002-7206-6266), Angus B MacKenzie, Gillian MacKinnon, Pauline Gulliver (0000-0003-1180-1578)
Year2015
Volume57
Issue3
Pages337-345
Publication date2015-01-01
Open AccessYes
TypeARTICLE
VenueRadiocarbon (JOURNAL)
Journal identifiersISSN: 0033-8222 • E-ISSN: 1945-5755
PublisherCambridge University Press (CUP) (PUBLISHER)
DOI10.2458/azu_rc.57.18395
OpenAlexW2049129590
LanguageEN
Citations received1
References cited16

During the period from 1995 to 2011, radiocarbon measurements from the coast around Hartlepool in NE England have revealed anomalous enrichments in seawater, sediment, and marine biota. These cannot be explained on the basis of atomic weapons testing or authorized nuclear industry discharges, including those from the nearby advanced gas-cooled reactor. Enhanced 14 C-specific activities have also been observed since 2005 in biota during routine monitoring at Hartlepool by the Food Standards Agency, but are reported as “likely” originating from a “nearby non-nuclear source.” Studies undertaken in Hartlepool and Teesmouth during 2005 and 2011 suggest that the 14 C discharges are in the vicinity of Greatham Creek, with activity levels in biota analogous to those measured at Sellafield, which discharges TBq activities of 14 C per annum. However, if the discharges are into Greatham Creek or even the River Tees, it is proposed that they would be much smaller than those at Sellafield and the high specific activities would be due to much smaller dilution factors. The discharge form of the 14 C remains unclear. The activity patterns in biota are similar to those at Sellafield, suggesting that initial inputs are dissolved inorganic carbon (DI 14 C). However, the mussel/seaweed ratios are more akin to those found around Amersham International, Cardiff, which is known to discharge 14 C in an organic form. 14 C analysis of a sediment core from Seal Sands demonstrated excess 14 C to the base of the core (43–44 cm). 210 Pb dating of the core (0–32 cm) produced an accumulation rate of 0.7 g cm −2 yr −1 , implying that 14 C discharges have occurred from the 1960s until the present day

Accelerator mass spectrometry · Biota · Carbon fibers · Dilution · Radiocarbon dating · Radionuclide · Seawater · Sediment · Chemistry · Environmental Science · Geology and Paleoclimatology Research · Isotope Analysis in Ecology · Radioactive contamination and transfer · Ecology · Environmental Chemistry · Geology · Oceanography · Paleontology

  • Experimental Investigation of 14C in the Primary Coolant of the 10 MW High Temperature Gas-Cooled Reactor

    Open Access•F Xie, W Peng et al.•Radiocarbon•2019

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    Open Access•Willem G Mook, Johannes Van Der Plicht•Radiocarbon•1999

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    Open Access•G T Cook, A B MACKENZIE et al.•Radiocarbon•2004

  • C AMS at Suerc

    Open Access•P Naysmith, G T Cook et al.•Radiocarbon•2010

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    Open Access•P Gulliver, G T Cook et al.•Radiocarbon•2004

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    Open Access•G T Cook, F H Begg et al.•Radiocarbon•1995

  • Anthropogenic Radiocarbon in the Eastern Irish Sea and Scottish Coastal Waters

    Open Access•F H Begg, G T Cook et al.•Radiocarbon•1992

Citations per year0.14
Citation span2019 - 2019 (1)
Highly citedNo

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