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Anthropogenic Rare Earth Elements

Gadolinium in a Small Catchment in Guizhou Province, Southwest China

Bibliographic Data

ID15514364
AuthorsJue Zhang (0000-0003-3427-3456, Guizhou University), Zhuhong Wang (Guiyang Medical University, corresponding author), Qixin Wu (0000-0002-4231-509X, Guizhou University, corresponding author), Yanling An (0000-0003-2351-615X, Guizhou Institute of Technology), Huipeng Jia (Guizhou University), Yuanyi Shen (Guizhou University)
Year2019
Volume16
Issue20
Pages4052-4052
Publication date2019-10-22
Open AccessYes
TypeARTICLE
VenueInternational Journal of Environmental Research and Public Health (JOURNAL)
Journal identifiersISSN: 1661-7827 • E-ISSN: 1660-4601
PublisherMultidisciplinary Digital Publishing Institute (PUBLISHER • CH)
DOI10.3390/ijerph16204052
PMID31652627
OpenAlexW2981943561
LanguageEN
Citations received2
References cited56

Rare earth elements (REEs), known as "industrial vitamins", are widely used in medical treatment, industry, agriculture, etc. However, with the increasing demand for REEs, excess REEs, such as gadolinium (Gd), are considered micropollutants in the environment. In this paper, the distributions of dissolved REEs were analyzed in three small streams, in order to determine the extent and occurrence of Gd anomalies. The shale-normalized REE patterns in the three streams were less smooth with heavy REEs higher than light REEs, for a weak reaction of the heavy REE complexes. A negative Ce (cerium) anomaly and positive samarium (Sm) and europium (Eu) anomalies were observed in the three streams and the negative Ce anomaly was affected by the pH of the alkaline rivers. However, a positive Gd anomaly was found in only a typical urban small stream, Jinzhong. With a population of approximately 60,000, Jinzhong runs by a hospital and through wastewater treatment plants (WWTPs). The concentrations of Gd in Jinzhong ranged from 1.54 to 86.65 ng/L with high anthropogenic Gd proportions (63.64%-98.07%). Anthropogenic Gd showed significant seasonal variations and distinct spatial disparities from upstream to downstream, and it was associated with certain ions such as Cl - . Anthropogenic Gd could be attributed to gadopentetic acid (Gd-DTPA), which is used in magnetic resonance imaging (MRI) in hospitals. This type of Gd was shown to be correlated with municipal wastewater. Due to the high stability and low particulate reactivity in water, anthropogenic Gd has great potential to serve as a tracer to prove the presence of medical wastewater

Archaeology · Cartography · Catchment area · China · Drainage basin · Earth science · Gadolinium · Geography · Physical geography · Rare earth · Chemistry · Environmental Science · Extraction and Separation Processes · Geochemistry and Elemental Analysis · Radioactive element chemistry and processing · Geology

  • Anthropogenic Gd in urban river water

    Open Access•Ruiyin Han, Zhuhong Wang et al.•Elementa Science of the…•2021

  • Distribution, water quality, and health risk assessment of trace elements in three streams during the wet season, Guiyang, Southwest China

    Open Access•Jue Zhang, Qixin Wu et al.•Elementa Science of the…•2021

  • Rare earth elements geochemistry in surface floodplain sediments from the Xiangjiang River, middle reach of Changjiang River, China

    Longjiang Mao, Duowen Mo et al.•Quaternary International•2014

Citations per year0.4
Citation span2021 - 2021 (1)
Highly citedNo

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