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The Radiocarbon Intracavity Optogalvanic Spectroscopy Setup at Uppsala

Dados Bibliográficos

ID9242192
AutoresGerriet Eilers, Anders Persson (0000-0001-7506-3899), Cecilia Gustavsson, Linus Ryderfors, Emad Mukhtar, Goran Possnert (0000-0002-4840-291X), Mehran Salehpour
Ano2013
Volume55
Fascículo2
Páginas237-250
Data de publicação2013-01-01
Peer ReviewedSim
Open AccessSim
TipoARTICLE
PeriódicoRadiocarbon (JOURNAL)
Identificadores do periódicoISSN: 0033-8222 • E-ISSN: 1945-5755
EditoraCambridge University Press (CUP) (PUBLISHER)
DOI10.1017/s0033822200057349
OpenAlexW4238533938
IdiomaEN
Citações recebidas2
Referências citadas12

Accelerator mass spectrometry (AMS) is by far the predominant technology deployed for radiocarbon tracer studies. Applications are widespread from archaeology to biological, environmental, and pharmaceutical sciences. In spite of its excellent performance, AMS is expensive and complicated to operate. Consequently, alternative detection techniques for 14 C are of great interest, with the vision of a compact, user-friendly, and inexpensive analytical method. Here, we report on the use of intracavity optogalvanic spectroscopy (ICOGS) for measurements of the 14 C/ 12 C ratio. This new detection technique was developed by Murnick et al. (2008). In the infrared (IR) region, CO 2 molecules have strong absorption coefficients. The IR-absorption lines are narrow in line width and shifted for different carbon isotopes. These properties can potentially be exploited to detect 14 CO 2 , 13 CO 2 , or 12 CO 2 molecules unambiguously. In ICOGS, the sample is in the form of CO 2 gas, eliminating the graphitization step that h is required in most AMS labs. The status of the ICOGS setup in Uppsala is presented. The system is operational but not yet fully developed. Data are presented for initial results that illustrate the dependence of the optogalvanic signal on various parameters, such as background and plasma-induced changes in the sample gas composition

Absorption spectroscopy · Accelerator mass spectrometry · Atomic physics · Carbon fibers · Infrared · Isotope · Isotopes of carbon · Mass spectrometry · Noble gas · Nuclear physics · Optics · Physics · Radiocarbon dating · TRACER · Atmospheric and Environmental Gas Dynamics · Atmospheric Ozone and Climate · Chemistry · Environmental Science · Materials Science · Spectroscopy and Laser Applications · Environmental Chemistry · Geology · Spectroscopy

  • Invalidation of the Intracavity Optogalvanic Method for Radiocarbon Detection

    Open Access•Cantwell G Carson, Martin Stute et al.•Radiocarbon•2016

Obras citantes distintas1
Citações por ano0,2
Intervalo de citações2016 - 2016 (1)
Velocidade de citaçãohistorical
Altamente citadoNão
Tipos de citaçãoNeutras: 2
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